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Using angle-resolved photoemission spectroscopy, we show direct evidence for charge transfer between adsorbed molecules and metal substrates, i.e., chemisorption of CO on Pt(111) and Pt–Sn/Pt(111) 2 × 2 surfaces. The observed band structures show a unique signature of charge transfer as CO atoms are adsorbed, revealing the roles of specific …
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An increase in the Sn/Pt ratio will further reduce the particle size of Pt and increase its dispersion. When the Sn/Pt ratio is 1.5, it shows the best catalytic activity. The metal particle size of the catalyst has a great influence on the dehydrogenation process of methylcyclopentane (MCP), showing an obvious size effect.
Although Pt-Sn catalyst supported over Beta zeolite with low acidity showed low Pt dispersion, it formed a relatively lower amount of coke on PDH reaction and maintained a high surface area and active Pt surfaces, resulting in enhanced stability for PDH reaction. This work can provide a better understanding of zeolite-supported Pt-Sn …
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2.1 Catalyst Preparation. SiO 2 supported Pt–Sn bimetallic catalysts were prepared via impregnation method with different synthesis procedures, as shown in Scheme 1.Prior to impregnation, the silica (JRC-SIO-9) was thermally treated in air at 773 K for 3 h. The pretreated SiO 2 support was then added into an aqueous solution of H 2 PtCl 6 6H …
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This study is aimed at investigating the impact of catalyst preparation's approach (either sequential and/or simultaneous wet impregnation) to a mesoporous series of Pt/A, Sn/A, PtSn/A, SnPt/A, (PtSn)/A, (PtSn)Zn/A, and (PtSnZn)/A catalysts for direct ethane dehydrogenation. The (PtSn)/A and (PtSnZn)/A had shown both higher initial …
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Propane dehydrogenation on Pt–Sn/Al 2 O 3 and Pt–Sn/ZnAl 2 O 4 was performed, and the Pt–Sn/ZnAl 2 O 4 catalyst showed a stronger tolerance for catalytic deactivation than the Pt–Sn/Al 2 O 3 catalyst. In this study, we propose that the high catalytic stability of Pt–Sn/ZnAl 2 O 4 originates from the relatively faster coke mobility …
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